The vibrational motions are usually neglected when calculating(e,2e) triple differential cross sections(TDCSs) of molecules. Here, multi-center distorted-wave method(MCDW) has been modified by including molecular vibrations. This vibrational MCDW method is employed to calculate the TDCSs of 1b3gorbital of ethylene at low(100 eV) and medium(250 eV) incident electron energies in coplanar asymmetric kinematic condition. The results show that molecular vibrations significantly influence the angular distributions of the TDCSs, especially in the binary region along momentum transfer near the Bethe ridge.
We report theoretical studies of electron impact triple differential cross sections of two bio-molecules,pyrimidine and tetrahydrofurfuryl alcohol,in the coplanar asymmetric kinematic conditions with the impact energy of 250 eV and ejected electron energy of 20 eV at three scattering angles of-5°,-10°,and-15°.Present multi-center distorted-wave method well describes theexperimental data,which was obtained by performing(e,2e)experiment.The calculations show that the secondary electron produced by the primary impact electron is strongly influenced by the molecular ionic multi-center potential,which must be considered when the low energy electron interacts with DNA analogues.
本文使用扭曲波波恩近似方法(DWBA)研究了共面对称条件下钙原子的电子碰撞电离反应((e,2e)反应),在DWBA理论的基础上,考虑了原子极化势和离子极化势对三重微分散射截面的影响.采用发展的DWBA方法,我们研究了出射电子能量从6.75 e V到29.25 e V范围内电子与钙原子的碰撞电离过程,计算了电离三重微分截面.通过与已有理论和实验数据进行比较发现,离子极化势对钙原子的共面对称(e,2e)反应散射微分截面有较大的影响,很好的描述了碰撞电离微分截面的结构效应,特别是在散射角度较小时(≦60o),本文计算结果与实验测量非常一致.
